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Key Points Modeled dissolved organic carbon export was 18.4 Tg C yr ‐1 (median) from 1982‐2019 for the six largest Arctic Rivers Proportional contributions of chromophoric to total dissolved organic carbon (CDOC & DOC) are positively correlated with water discharge Increasing discharge and shifting seasonality, independent of other factors, would have increased CDOC and DOC export from 1982‐2019 

Arctic rivers provide an integrated signature of the changing landscape and transmit signals of change to the ocean. Here, we use a decade of particulate organic matter (POM) compositional data to deconvolute multiple allochthonous and autochthonous pan-Arctic and watershed-specific sources. Constraints from carbon-to-nitrogen ratios (C:N), δ 13 C, and Δ 14 C signatures reveal a large, hitherto overlooked contribution from aquatic biomass. Separation in Δ 14 C age is enhanced by splitting soil sources into shallow and deep pools (mean ± SD: −228 ± 211 vs. −492 ± 173‰) rather than traditional active layer and permafrost pools (−300 ± 236 vs. −441 ± 215‰) that do not represent permafrost-free Arctic regions. We estimate that 39 to 60% (5 to 95% credible interval) of the annual pan-Arctic POM flux (averaging 4,391 Gg/y particulate organic carbon from 2012 to 2019) comes from aquatic biomass. The remainder is sourced from yedoma, deep soils, shallow soils, petrogenic inputs, and fresh terrestrial production. Climate change-induced warming and increasing CO 2 concentrations may enhance both soil destabilization and Arctic river aquatic biomass production, increasing fluxes of POM to the ocean. Younger, autochthonous, and older soil-derived POM likely have different destinies (preferential microbial uptake and processing vs. significant sediment burial, respectively). A small (~7%) increase in aquatic biomass POM flux with warming would be equivalent to a ~30% increase in deep soil POM flux. There is a clear need to better quantify how the balance of endmember fluxes may shift with different ramifications for different endmembers and how this will impact the Arctic system. 

Northern regions are undergoing rapid change with wildfires increasing in frequency and severity alongside thawing permafrost and altered water balance. These disturbances could cause significant change in the export of carbon, nutrients, and metals to aquatic systems, with implications for food webs and ecosystem processes. Here, we examine chemical data from a series of 52 streams and rivers that were sampled across a 250,000 km²expanse of the Taiga Plains and Taiga Shield ecozones of the Northwest Territories, Canada. Samples were collected immediately after and for 3 years following a “megafire” that occurred in this region in 2014, and included wildfire‐affected and non‐affected catchments. While wildfire has been observed to cause significant impacts on water quality in other regions, we here report weak relationships with percent watershed burn with minor to moderate effect sizes, the greatest being a reduction in dissolved organic carbon (−32% concentration). Watershed‐specific properties were a strong driver of large spatial variability in stream water chemistry, which may overwhelm or obscure lesser wildfire effects. The watershed chemical yield‐specific response to wildfire was weaker than the response for concentrations, due to substantial variation and uncertainty in runoff among sites and years. This suggests that watershed chemical yields in this region are more sensitive to changes in water balance due to climate than to altered wildfire regimes.

 

High levels of methylmercury accumulation in marine biota are a concern throughout the Arctic, where coastal ocean ecosystems received large riverine inputs of mercury (Hg) (40 Mg⋅y −1 ) and sediment (20 Tg⋅y −1 ) during the last decade, primarily from major Russian rivers. Hg concentrations in fish harvested from these rivers have declined since the late 20th century, but no temporal data on riverine Hg, which is often strongly associated with suspended sediments, were previously available. Here, we investigate temporal trends in Russian river particulate Hg (PHg) and total suspended solids (TSS) to better understand recent changes in the Arctic Hg cycle and its potential future trajectories. We used 1,300 measurements of Hg in TSS together with discharge observations made by Russian hydrochemistry and hydrology monitoring programs to examine changes in PHg and TSS concentrations and fluxes in eight major Russian rivers between ca. 1975 and 2010. Due to decreases in both PHg concentrations (micrograms per gram) and TSS loads, annual PHg export declined from 47 to 7 Mg⋅y −1 overall and up to 92% for individual rivers. Modeling of atmospheric Hg deposition together with published inventories on reservoir establishment and industrial Hg release point to decreased pollution and sedimentation within reservoirs as predominant drivers of declining PHg export. We estimate that Russian rivers were the primary source of Hg to the Arctic Ocean in the mid to late 20th century. 

Climate change is an existential threat to the vast global permafrost domain. The diverse human cultures, ecological communities, and biogeochemical cycles of this tenth of the planet depend on the persistence of frozen conditions. The complexity, immensity, and remoteness of permafrost ecosystems make it difficult to grasp how quickly things are changing and what can be done about it. Here, we summarize terrestrial and marine changes in the permafrost domain with an eye toward global policy. While many questions remain, we know that continued fossil fuel burning is incompatible with the continued existence of the permafrost domain as we know it. If we fail to protect permafrost ecosystems, the consequences for human rights, biosphere integrity, and global climate will be severe. The policy implications are clear: the faster we reduce human emissions and draw down atmospheric CO 2 , the more of the permafrost domain we can save. Emissions reduction targets must be strengthened and accompanied by support for local peoples to protect intact ecological communities and natural carbon sinks within the permafrost domain. Some proposed geoengineering interventions such as solar shading, surface albedo modification, and vegetation manipulations are unproven and may exacerbate environmental injustice without providing lasting protection. Conversely, astounding advances in renewable energy have reopened viable pathways to halve human greenhouse gas emissions by 2030 and effectively stop them well before 2050. We call on leaders, corporations, researchers, and citizens everywhere to acknowledge the global importance of the permafrost domain and work towards climate restoration and empowerment of Indigenous and immigrant communities in these regions.